Independent magnon states on magnetic polytopes

For many spin systems with constant isotropic antiferromagnetic next-neighbour Heisenberg coupling the minimal energies E_{min}(S) form a rotational band, i.e. depend approximately quadratically on the total spin quantum number S, a property which is also known as Lande interval rule. However, we find that for certain coupling topologies, including recently synthesised icosidodecahedral structures this rule is violated for high total spins. Instead the minimal energies are a linear function of total spin. This anomaly results in a corresponding jump of the magnetisation curve which otherwise would be a regular staircase.Comment: 11 pages, 4 figures, submitted to Eur. Phys. J.

Non-rigid hole band in the extended t-J model

The dispersion of one hole in an extended $t$-$J$ model with additional hopping terms to second and third nearest neighbours and a frustration term in the exchange part has been investigated. Two methods, a Green's function projection technique describing a magnetic polaron of minimal size and the exact diagonalization of a $4*4$ lattice, have been applied, showing reasonable agreement among each other. Using additional hopping integrals which are characteristic for the CuO$_2$ plane in cuprates we find in the nonfrustrated case an isotropic minimum of the dispersion at the point $(\pi/2,\pi/2)$ in $k$-space in good coincidence with recent angle-resolved photoemission results for the insulating compound Sr$_2$CuO$_2$Cl$_2$. Including frustration or finite temperature which shall simulate the effect of doping, the dispersion is drastically changed such that a flat region and an extended saddle point may be observed between $(\pi/2,0)$ and $(\pi,0)$ in agreement with experimental results for the optimally doped cuprates.Comment: 14 pages, LaTeX, 6 figures on request, submitted to Zeitschrift fuer Physi

Macroscopic magnetization jumps due to independent magnons in frustrated quantum spin lattices

For a class of frustrated spin lattices including the kagome lattice we construct exact eigenstates consisting of several independent, localized one-magnon states and argue that they are ground states for high magnetic fields. If the maximal number of local magnons scales with the number of spins in the system, which is the case for the kagome lattice, the effect persists in the thermodynamic limit and gives rise to a macroscopic jump in the zero-temperature magnetization curve just below the saturation field. The effect decreases with increasing spin quantum number and vanishes in the classical limit. Thus it is a true macroscopic quantum effect.Comment: 4 pages, 4 figures, accepted by Phys.Rev.Let

The DSUBmm Approximation Scheme for the Coupled Cluster Method and Applications to Quantum Magnets

A new approximate scheme, DSUB$m$, is described for the coupled cluster method. We then apply it to two well-studied (spin-1/2 Heisenberg antiferromagnet) spin-lattice models, namely: the $XXZ$ and the $XY$ models on the square lattice in two dimensions. Results are obtained in each case for the ground-state energy, the sublattice magnetization and the quantum critical point. They are in good agreement with those from such alternative methods as spin-wave theory, series expansions, quantum Monte Carlo methods and those from the CCM using the LSUB$m$ scheme.Comment: 18 pages, 10 figure

Ground state and low-lying excitations of the spin-1/2 XXZ model on the kagome lattice at magnetization 1/3

We study the ground state and low-lying excitations of the S=1/2 XXZ antiferromagnet on the kagome lattice at magnetization one third of the saturation. An exponential number of non-magnetic states is found below a magnetic gap. The non-magnetic excitations also have a gap above the ground state, but it is much smaller than the magnetic gap. This ground state corresponds to an ordered pattern with resonances in one third of the hexagons. The spin-spin correlation function is short ranged, but there is long-range order of valence-bond crystal type.Comment: 2 pages, 1 figure included, to appear in Physica B (proceedings of SCES'04

Diamond chains with multiple-spin exchange interactions

We study the phase diagram of a symmetric spin-1/2 Heisenberg diamond chain with additional cyclic four-spin exchange interactions. The presented analysis supplemented by numerical exact-diagonalization results for finite periodic clusters implies a rich phase diagram containing, apart from standard magnetic and spin-liquid phases, two different tetramer-dimer phases as well as an exotic four-fold degenerate dimerized phase. The characteristics of the established spin phases as well as the nature of quantum phase transitions are discussed, as well.Comment: 6 PRB pages, Added reference

Frustration effects in magnetic molecules

By means of exact diagonalization we study the ground-state and the low-temperature physics of the Heisenberg antiferromagnet on the cuboctahedron and the icosidodecahedron. Both are frustrated magnetic polytopes and correspond to the arrangement of magnetic atoms in the magnetic molecules Cu12La8 and Mo72Fe30. The interplay of strong quantum fluctuations and frustration influences the ground state spin correlations drastically and leads to an interesting magnetization process at low temperatures. Furthermore the frustration yields low-lying non-magnetic excitations resulting in an extra low-temperature peak in the specific heat.Comment: 4 pages, 7 figure